Abstract

Transition metal dichalcogenides (TMDCs), belonging to the class of van der Waals materials, are promising materials for optoelectronics and photonics. In particular, their giant optical anisotropy may enable important optical effects when employed in nanostructures with finite thickness. In this paper, we theoretically and numerically study light scattering behavior from anisotropic MoS₂ nanocylinders, and highlight its distinct features advantageous over the response of conventional silicon particles of the same shape. We establish two remarkable phenomena, appearing in the same MoS₂ particle with optimized geometry. The first one is a pure magnetic dipole scattering associated with the excitation of the electric-dipole anapole states. Previously reported in core-shell hybrid (metal/dielectric) systems only, it is now demonstrated in an all-dielectric particle. The second phenomenon is the super-deflection in the far field: the maximum scattering may occur over a wide range of directions, including forward-, backward- and side-scattering depending on the mutual orientation of the MoS₂ nanocylinder and the incident wave. In contrast to the well-known Kerker and anti-Kerker effects, which appear in nanoparticles at different frequencies, the super-deflection can be achieved by rotating the particle at a constant frequency of incident light. Our results facilitate the development of functional optical devices incorporating nanostructured anisotropic TMDCs and may encourage further research in meta-optics based on highly anisotropic materials.

Abstract

Transition metal dichalcogenides (TMDCs), belonging to the class of van der Waals materials, are promising materials for optoelectronics and photonics. In particular, their giant optical anisotropy may enable important optical effects when employed in nanostructures with finite thickness. In this paper, we theoretically and numerically study light scattering behavior from anisotropic MoS₂ nanocylinders, and highlight its distinct features advantageous over the response of conventional silicon particles of the same shape. We establish two remarkable phenomena, appearing in the same MoS₂ particle with optimized geometry. The first one is a pure magnetic dipole scattering associated with the excitation of the electric-dipole anapole states. Previously reported in core-shell hybrid (metal/dielectric) systems only, it is now demonstrated in an all-dielectric particle. The second phenomenon is the super-deflection in the far field: the maximum scattering may occur over a wide range of directions, including forward-, backward- and side-scattering depending on the mutual orientation of the MoS₂ nanocylinder and the incident wave. In contrast to the well-known Kerker and anti-Kerker effects, which appear in nanoparticles at different frequencies, the super-deflection can be achieved by rotating the particle at a constant frequency of incident light. Our results facilitate the development of functional optical devices incorporating nanostructured anisotropic TMDCs and may encourage further research in meta-optics based on highly anisotropic materials.

Abstract

Transition metal dichalcogenides (TMDCs), belonging to the class of van der Waals materials, are promising materials for optoelectronics and photonics. In particular, their giant optical anisotropy may enable important optical effects when employed in nanostructures with finite thickness. In this paper, we theoretically and numerically study light scattering behavior from anisotropic MoS₂ nanocylinders, and highlight its distinct features advantageous over the response of conventional silicon particles of the same shape. We establish two remarkable phenomena, appearing in the same MoS₂ particle with optimized geometry. The first one is a pure magnetic dipole scattering associated with the excitation of the electric-dipole anapole states. Previously reported in core-shell hybrid (metal/dielectric) systems only, it is now demonstrated in an all-dielectric particle. The second phenomenon is the super-deflection in the far field: the maximum scattering may occur over a wide range of directions, including forward-, backward- and side-scattering depending on the mutual orientation of the MoS₂ nanocylinder and the incident wave. In contrast to the well-known Kerker and anti-Kerker effects, which appear in nanoparticles at different frequencies, the super-deflection can be achieved by rotating the particle at a constant frequency of incident light. Our results facilitate the development of functional optical devices incorporating nanostructured anisotropic TMDCs and may encourage further research in meta-optics based on highly anisotropic materials.

Abstract

Transition metal dichalcogenides (TMDCs), belonging to the class of van der Waals materials, are promising materials for optoelectronics and photonics. In particular, their giant optical anisotropy may enable important optical effects when employed in nanostructures with finite thickness. In this paper, we theoretically and numerically study light scattering behavior from anisotropic MoS₂ nanocylinders, and highlight its distinct features advantageous over the response of conventional silicon particles of the same shape. We establish two remarkable phenomena, appearing in the same MoS₂ particle with optimized geometry. The first one is a pure magnetic dipole scattering associated with the excitation of the electric-dipole anapole states. Previously reported in core-shell hybrid (metal/dielectric) systems only, it is now demonstrated in an all-dielectric particle. The second phenomenon is the super-deflection in the far field: the maximum scattering may occur over a wide range of directions, including forward-, backward- and side-scattering depending on the mutual orientation of the MoS₂ nanocylinder and the incident wave. In contrast to the well-known Kerker and anti-Kerker effects, which appear in nanoparticles at different frequencies, the super-deflection can be achieved by rotating the particle at a constant frequency of incident light. Our results facilitate the development of functional optical devices incorporating nanostructured anisotropic TMDCs and may encourage further research in meta-optics based on highly anisotropic materials.