Abstract

We analyse in this article the many-body behavior of free-standing doped graphene nanoribbons where the chemical potential lies inside the bulk single-particle bands. We perform an exact mapping from both an extended and an on-site Hubbard model of the ribbons to a Kanamori model, which includes ferromagnetic exchange and pair-hopping interactions. We determine the resulting Coulomb matrix elements analytically, and identify their scaling behavior as a function of ribbon width and length. We propose a low-energy version of the Kanamori Hamiltonian to address the response of the ribbons to external fields, with a view to their use as transport channels in nanoelectronics. We find that the model and the proposed ribbon parameters can produce open-shell, high-spin many-body states that can lead to shell- and spin-blockade responses.

Abstract

We analyse in this article the many-body behavior of free-standing doped graphene nanoribbons where the chemical potential lies inside the bulk single-particle bands. We perform an exact mapping from both an extended and an on-site Hubbard model of the ribbons to a Kanamori model, which includes ferromagnetic exchange and pair-hopping interactions. We determine the resulting Coulomb matrix elements analytically, and identify their scaling behavior as a function of ribbon width and length. We propose a low-energy version of the Kanamori Hamiltonian to address the response of the ribbons to external fields, with a view to their use as transport channels in nanoelectronics. We find that the model and the proposed ribbon parameters can produce open-shell, high-spin many-body states that can lead to shell- and spin-blockade responses.

Abstract

We analyse in this article the many-body behavior of free-standing doped graphene nanoribbons where the chemical potential lies inside the bulk single-particle bands. We perform an exact mapping from both an extended and an on-site Hubbard model of the ribbons to a Kanamori model, which includes ferromagnetic exchange and pair-hopping interactions. We determine the resulting Coulomb matrix elements analytically, and identify their scaling behavior as a function of ribbon width and length. We propose a low-energy version of the Kanamori Hamiltonian to address the response of the ribbons to external fields, with a view to their use as transport channels in nanoelectronics. We find that the model and the proposed ribbon parameters can produce open-shell, high-spin many-body states that can lead to shell- and spin-blockade responses.

Abstract

We analyse in this article the many-body behavior of free-standing doped graphene nanoribbons where the chemical potential lies inside the bulk single-particle bands. We perform an exact mapping from both an extended and an on-site Hubbard model of the ribbons to a Kanamori model, which includes ferromagnetic exchange and pair-hopping interactions. We determine the resulting Coulomb matrix elements analytically, and identify their scaling behavior as a function of ribbon width and length. We propose a low-energy version of the Kanamori Hamiltonian to address the response of the ribbons to external fields, with a view to their use as transport channels in nanoelectronics. We find that the model and the proposed ribbon parameters can produce open-shell, high-spin many-body states that can lead to shell- and spin-blockade responses.